Physics of structured light, matter and their interactions

Nonlinear Spectroscopy and Structured Matter

SLAM research overview

We use ultrafast, high-intensity laser pulses to investigate nonlinear light–matter interactions in spatially structured and complex materials.

Group leader: Domenico Paparo
A research group within the SLAM cluster

We combine femtosecond lasers, nonlinear frequency conversion and intense terahertz (THz) pulses to study soft and condensed matter. Nonlinear optical techniques provide sensitivity to surfaces and interfaces and reveal material dynamics across a broad spectral range.

Schematic of coherent terahertz hyper-Raman spectroscopy showing infrared and terahertz fields, a sample and the detected optical signal
Concept of coherent terahertz hyper-Raman spectroscopy: an intense THz field drives a nonlinear material response that is read out through an optical signal.

Research lines

Surface and interface spectroscopy

We exploit second-order nonlinear processes, including second-harmonic generation, to probe surface and interface properties with sub-nanometre sensitivity.

Broadband terahertz generation

We use two-colour four-wave mixing in air to generate intense, broadband, single-cycle terahertz pulses for time-resolved spectroscopy.

Nonlinear THz phenomena

We investigate nonlinear responses driven by intense THz fields, including coherent THz hyper-Raman spectroscopy, in which the material response is read out optically.

Structured ultrafast fields

We develop spatially structured ultrafast pulses and study how their tailored amplitude, phase and polarization influence light–matter interactions.

Materials and systems

Our studies span heterostructures of strongly correlated transition-metal oxides, ultrathin ferroelectric films, laser-treated diamond for THz applications and ionic liquids.

Explore SLAM

This group is part of SLAM, a cluster of three independent research groups with shared scientific interests and resources.